Hyperfine interactions at ¹⁸¹Hf(→¹⁸¹Ta) impurities implanted in Er₂O₃ and Gd₂O₃: structural and electronic dependence of the EFG in bixbyite sesquioxides

The time-differential-perturbed γ-γ angular-correlation technique (TDPAC) with ion-implanted ¹⁸¹Hf tracers has been applied to study the hyperfine interactions of ¹⁸¹Ta impurities in the cubic bixbyite structure of Er₂O₃ and Gd₂O₃. The TDPAC experiments were performed in air in the temperature range...

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Detalles Bibliográficos
Autores principales: Errico, Leonardo Antonio, Rentería, Mario, Pasquevich, Alberto Felipe, Bibiloni, Aníbal Guillermo, Freitag, Kristian
Formato: Articulo
Lenguaje:Inglés
Publicado: 2001
Materias:
Acceso en línea:http://sedici.unlp.edu.ar/handle/10915/146300
Aporte de:
id I19-R120-10915-146300
record_format dspace
institution Universidad Nacional de La Plata
institution_str I-19
repository_str R-120
collection SEDICI (UNLP)
language Inglés
topic Ciencias Exactas
Física
Doping and impurity implantation in other materials
Mössbauer effect; other gamma-ray spectroscopy
Nuclear states and interactions
spellingShingle Ciencias Exactas
Física
Doping and impurity implantation in other materials
Mössbauer effect; other gamma-ray spectroscopy
Nuclear states and interactions
Errico, Leonardo Antonio
Rentería, Mario
Pasquevich, Alberto Felipe
Bibiloni, Aníbal Guillermo
Freitag, Kristian
Hyperfine interactions at ¹⁸¹Hf(→¹⁸¹Ta) impurities implanted in Er₂O₃ and Gd₂O₃: structural and electronic dependence of the EFG in bixbyite sesquioxides
topic_facet Ciencias Exactas
Física
Doping and impurity implantation in other materials
Mössbauer effect; other gamma-ray spectroscopy
Nuclear states and interactions
description The time-differential-perturbed γ-γ angular-correlation technique (TDPAC) with ion-implanted ¹⁸¹Hf tracers has been applied to study the hyperfine interactions of ¹⁸¹Ta impurities in the cubic bixbyite structure of Er₂O₃ and Gd₂O₃. The TDPAC experiments were performed in air in the temperature range 300-1073 K (in the case of Er₂O₃) and 300-1173 K (in the case of Gd₂O₃). Three electrical-quadrupole interactions were found in each oxide in the whole studied temperature range. Two of them were attributed to the electric-field gradients (EFG) acting on ¹⁸¹Ta probes substitutionally located on the two nonequivalent free-of-defects cation sites of the bixbyite structure. The EFG results are compared with predictions of the point-charge model and discussed together with previous results obtained with the probes ¹¹¹Cd and ¹⁸¹Ta in other isomorphous sesquioxides. The temperature dependence of the hyperfine parameters for both oxides is also discussed in terms of dilatometric expansion data.
format Articulo
Articulo
author Errico, Leonardo Antonio
Rentería, Mario
Pasquevich, Alberto Felipe
Bibiloni, Aníbal Guillermo
Freitag, Kristian
author_facet Errico, Leonardo Antonio
Rentería, Mario
Pasquevich, Alberto Felipe
Bibiloni, Aníbal Guillermo
Freitag, Kristian
author_sort Errico, Leonardo Antonio
title Hyperfine interactions at ¹⁸¹Hf(→¹⁸¹Ta) impurities implanted in Er₂O₃ and Gd₂O₃: structural and electronic dependence of the EFG in bixbyite sesquioxides
title_short Hyperfine interactions at ¹⁸¹Hf(→¹⁸¹Ta) impurities implanted in Er₂O₃ and Gd₂O₃: structural and electronic dependence of the EFG in bixbyite sesquioxides
title_full Hyperfine interactions at ¹⁸¹Hf(→¹⁸¹Ta) impurities implanted in Er₂O₃ and Gd₂O₃: structural and electronic dependence of the EFG in bixbyite sesquioxides
title_fullStr Hyperfine interactions at ¹⁸¹Hf(→¹⁸¹Ta) impurities implanted in Er₂O₃ and Gd₂O₃: structural and electronic dependence of the EFG in bixbyite sesquioxides
title_full_unstemmed Hyperfine interactions at ¹⁸¹Hf(→¹⁸¹Ta) impurities implanted in Er₂O₃ and Gd₂O₃: structural and electronic dependence of the EFG in bixbyite sesquioxides
title_sort hyperfine interactions at ¹⁸¹hf(→¹⁸¹ta) impurities implanted in er₂o₃ and gd₂o₃: structural and electronic dependence of the efg in bixbyite sesquioxides
publishDate 2001
url http://sedici.unlp.edu.ar/handle/10915/146300
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