Hyperfine interactions at ¹⁸¹Hf(→¹⁸¹Ta) impurities implanted in Er₂O₃ and Gd₂O₃: structural and electronic dependence of the EFG in bixbyite sesquioxides
The time-differential-perturbed γ-γ angular-correlation technique (TDPAC) with ion-implanted ¹⁸¹Hf tracers has been applied to study the hyperfine interactions of ¹⁸¹Ta impurities in the cubic bixbyite structure of Er₂O₃ and Gd₂O₃. The TDPAC experiments were performed in air in the temperature range...
Autores principales: | , , , , |
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Formato: | Articulo |
Lenguaje: | Inglés |
Publicado: |
2001
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Acceso en línea: | http://sedici.unlp.edu.ar/handle/10915/146300 |
Aporte de: |
id |
I19-R120-10915-146300 |
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record_format |
dspace |
institution |
Universidad Nacional de La Plata |
institution_str |
I-19 |
repository_str |
R-120 |
collection |
SEDICI (UNLP) |
language |
Inglés |
topic |
Ciencias Exactas Física Doping and impurity implantation in other materials Mössbauer effect; other gamma-ray spectroscopy Nuclear states and interactions |
spellingShingle |
Ciencias Exactas Física Doping and impurity implantation in other materials Mössbauer effect; other gamma-ray spectroscopy Nuclear states and interactions Errico, Leonardo Antonio Rentería, Mario Pasquevich, Alberto Felipe Bibiloni, Aníbal Guillermo Freitag, Kristian Hyperfine interactions at ¹⁸¹Hf(→¹⁸¹Ta) impurities implanted in Er₂O₃ and Gd₂O₃: structural and electronic dependence of the EFG in bixbyite sesquioxides |
topic_facet |
Ciencias Exactas Física Doping and impurity implantation in other materials Mössbauer effect; other gamma-ray spectroscopy Nuclear states and interactions |
description |
The time-differential-perturbed γ-γ angular-correlation technique (TDPAC) with ion-implanted ¹⁸¹Hf tracers has been applied to study the hyperfine interactions of ¹⁸¹Ta impurities in the cubic bixbyite structure of Er₂O₃ and Gd₂O₃. The TDPAC experiments were performed in air in the temperature range 300-1073 K (in the case of Er₂O₃) and 300-1173 K (in the case of Gd₂O₃). Three electrical-quadrupole interactions were found in each oxide in the whole studied temperature range. Two of them were attributed to the electric-field gradients (EFG) acting on ¹⁸¹Ta probes substitutionally located on the two nonequivalent free-of-defects cation sites of the bixbyite structure. The EFG results are compared with predictions of the point-charge model and discussed together with previous results obtained with the probes ¹¹¹Cd and ¹⁸¹Ta in other isomorphous sesquioxides. The temperature dependence of the hyperfine parameters for both oxides is also discussed in terms of dilatometric expansion data. |
format |
Articulo Articulo |
author |
Errico, Leonardo Antonio Rentería, Mario Pasquevich, Alberto Felipe Bibiloni, Aníbal Guillermo Freitag, Kristian |
author_facet |
Errico, Leonardo Antonio Rentería, Mario Pasquevich, Alberto Felipe Bibiloni, Aníbal Guillermo Freitag, Kristian |
author_sort |
Errico, Leonardo Antonio |
title |
Hyperfine interactions at ¹⁸¹Hf(→¹⁸¹Ta) impurities implanted in Er₂O₃ and Gd₂O₃: structural and electronic dependence of the EFG in bixbyite sesquioxides |
title_short |
Hyperfine interactions at ¹⁸¹Hf(→¹⁸¹Ta) impurities implanted in Er₂O₃ and Gd₂O₃: structural and electronic dependence of the EFG in bixbyite sesquioxides |
title_full |
Hyperfine interactions at ¹⁸¹Hf(→¹⁸¹Ta) impurities implanted in Er₂O₃ and Gd₂O₃: structural and electronic dependence of the EFG in bixbyite sesquioxides |
title_fullStr |
Hyperfine interactions at ¹⁸¹Hf(→¹⁸¹Ta) impurities implanted in Er₂O₃ and Gd₂O₃: structural and electronic dependence of the EFG in bixbyite sesquioxides |
title_full_unstemmed |
Hyperfine interactions at ¹⁸¹Hf(→¹⁸¹Ta) impurities implanted in Er₂O₃ and Gd₂O₃: structural and electronic dependence of the EFG in bixbyite sesquioxides |
title_sort |
hyperfine interactions at ¹⁸¹hf(→¹⁸¹ta) impurities implanted in er₂o₃ and gd₂o₃: structural and electronic dependence of the efg in bixbyite sesquioxides |
publishDate |
2001 |
url |
http://sedici.unlp.edu.ar/handle/10915/146300 |
work_keys_str_mv |
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Repositorios |
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1764820460947636227 |