Hyperfine interactions at ¹⁸¹Hf(→¹⁸¹Ta) impurities implanted in Er₂O₃ and Gd₂O₃: structural and electronic dependence of the EFG in bixbyite sesquioxides
The time-differential-perturbed γ-γ angular-correlation technique (TDPAC) with ion-implanted ¹⁸¹Hf tracers has been applied to study the hyperfine interactions of ¹⁸¹Ta impurities in the cubic bixbyite structure of Er₂O₃ and Gd₂O₃. The TDPAC experiments were performed in air in the temperature range...
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| Autores principales: | , , , , |
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| Formato: | Articulo |
| Lenguaje: | Inglés |
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2001
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| Acceso en línea: | http://sedici.unlp.edu.ar/handle/10915/146300 |
| Aporte de: |
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I19-R120-10915-146300 |
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dspace |
| institution |
Universidad Nacional de La Plata |
| institution_str |
I-19 |
| repository_str |
R-120 |
| collection |
SEDICI (UNLP) |
| language |
Inglés |
| topic |
Ciencias Exactas Física Doping and impurity implantation in other materials Mössbauer effect; other gamma-ray spectroscopy Nuclear states and interactions |
| spellingShingle |
Ciencias Exactas Física Doping and impurity implantation in other materials Mössbauer effect; other gamma-ray spectroscopy Nuclear states and interactions Errico, Leonardo Antonio Rentería, Mario Pasquevich, Alberto Felipe Bibiloni, Aníbal Guillermo Freitag, Kristian Hyperfine interactions at ¹⁸¹Hf(→¹⁸¹Ta) impurities implanted in Er₂O₃ and Gd₂O₃: structural and electronic dependence of the EFG in bixbyite sesquioxides |
| topic_facet |
Ciencias Exactas Física Doping and impurity implantation in other materials Mössbauer effect; other gamma-ray spectroscopy Nuclear states and interactions |
| description |
The time-differential-perturbed γ-γ angular-correlation technique (TDPAC) with ion-implanted ¹⁸¹Hf tracers has been applied to study the hyperfine interactions of ¹⁸¹Ta impurities in the cubic bixbyite structure of Er₂O₃ and Gd₂O₃. The TDPAC experiments were performed in air in the temperature range 300-1073 K (in the case of Er₂O₃) and 300-1173 K (in the case of Gd₂O₃). Three electrical-quadrupole interactions were found in each oxide in the whole studied temperature range. Two of them were attributed to the electric-field gradients (EFG) acting on ¹⁸¹Ta probes substitutionally located on the two nonequivalent free-of-defects cation sites of the bixbyite structure. The EFG results are compared with predictions of the point-charge model and discussed together with previous results obtained with the probes ¹¹¹Cd and ¹⁸¹Ta in other isomorphous sesquioxides. The temperature dependence of the hyperfine parameters for both oxides is also discussed in terms of dilatometric expansion data. |
| format |
Articulo Articulo |
| author |
Errico, Leonardo Antonio Rentería, Mario Pasquevich, Alberto Felipe Bibiloni, Aníbal Guillermo Freitag, Kristian |
| author_facet |
Errico, Leonardo Antonio Rentería, Mario Pasquevich, Alberto Felipe Bibiloni, Aníbal Guillermo Freitag, Kristian |
| author_sort |
Errico, Leonardo Antonio |
| title |
Hyperfine interactions at ¹⁸¹Hf(→¹⁸¹Ta) impurities implanted in Er₂O₃ and Gd₂O₃: structural and electronic dependence of the EFG in bixbyite sesquioxides |
| title_short |
Hyperfine interactions at ¹⁸¹Hf(→¹⁸¹Ta) impurities implanted in Er₂O₃ and Gd₂O₃: structural and electronic dependence of the EFG in bixbyite sesquioxides |
| title_full |
Hyperfine interactions at ¹⁸¹Hf(→¹⁸¹Ta) impurities implanted in Er₂O₃ and Gd₂O₃: structural and electronic dependence of the EFG in bixbyite sesquioxides |
| title_fullStr |
Hyperfine interactions at ¹⁸¹Hf(→¹⁸¹Ta) impurities implanted in Er₂O₃ and Gd₂O₃: structural and electronic dependence of the EFG in bixbyite sesquioxides |
| title_full_unstemmed |
Hyperfine interactions at ¹⁸¹Hf(→¹⁸¹Ta) impurities implanted in Er₂O₃ and Gd₂O₃: structural and electronic dependence of the EFG in bixbyite sesquioxides |
| title_sort |
hyperfine interactions at ¹⁸¹hf(→¹⁸¹ta) impurities implanted in er₂o₃ and gd₂o₃: structural and electronic dependence of the efg in bixbyite sesquioxides |
| publishDate |
2001 |
| url |
http://sedici.unlp.edu.ar/handle/10915/146300 |
| work_keys_str_mv |
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Repositorios |
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