Efficient energy transfer in layered hybrid organic/inorganic nanocomposites: A dual function of semiconductor nanocrystals
The efficiency of energy transfer in hybrid organic/inorganic nanocomposites based on conjugated polymers and semiconductor nanocrystals is strongly dependent on both the energy transfer rate and the rate of the nonradiative recombination of the polymer. We demonstrate that the polymer nonradiative...
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todo:paper_00036951_v96_n8_p_Lutich2023-10-03T13:56:37Z Efficient energy transfer in layered hybrid organic/inorganic nanocomposites: A dual function of semiconductor nanocrystals Lutich, A.A. Pöschl, A. Jiang, G. Stefani, F.D. Susha, A.S. Rogach, A.L. Feldmann, J. CdTe nanocrystals Dual function Dual role Efficiency of energy transfer Efficient energy transfer Energy-transfer rate Exciton diffusion Hybrid structure Layer-by-layers Non-radiative recombinations Organic/inorganic nano-composite Semiconductor nanocrystals Cadmium compounds Energy transfer Excitons Nanocomposites Nanocrystals Conjugated polymers The efficiency of energy transfer in hybrid organic/inorganic nanocomposites based on conjugated polymers and semiconductor nanocrystals is strongly dependent on both the energy transfer rate and the rate of the nonradiative recombination of the polymer. We demonstrate that the polymer nonradiative recombination can be reduced by the suppression of exciton diffusion via proper morphology engineering of a hybrid structure. In the layer-by-layer assembled nanocomposite of a conjugated polymer and CdTe nanocrystals the latter have a dual role: first, they are efficient exciton acceptors and, second, they reduce nonradiative recombination in the polymer by suppressing exciton diffusion across the layers. © 2010 American Institute of Physics. JOUR info:eu-repo/semantics/openAccess http://creativecommons.org/licenses/by/2.5/ar http://hdl.handle.net/20.500.12110/paper_00036951_v96_n8_p_Lutich |
| institution |
Universidad de Buenos Aires |
| institution_str |
I-28 |
| repository_str |
R-134 |
| collection |
Biblioteca Digital - Facultad de Ciencias Exactas y Naturales (UBA) |
| topic |
CdTe nanocrystals Dual function Dual role Efficiency of energy transfer Efficient energy transfer Energy-transfer rate Exciton diffusion Hybrid structure Layer-by-layers Non-radiative recombinations Organic/inorganic nano-composite Semiconductor nanocrystals Cadmium compounds Energy transfer Excitons Nanocomposites Nanocrystals Conjugated polymers |
| spellingShingle |
CdTe nanocrystals Dual function Dual role Efficiency of energy transfer Efficient energy transfer Energy-transfer rate Exciton diffusion Hybrid structure Layer-by-layers Non-radiative recombinations Organic/inorganic nano-composite Semiconductor nanocrystals Cadmium compounds Energy transfer Excitons Nanocomposites Nanocrystals Conjugated polymers Lutich, A.A. Pöschl, A. Jiang, G. Stefani, F.D. Susha, A.S. Rogach, A.L. Feldmann, J. Efficient energy transfer in layered hybrid organic/inorganic nanocomposites: A dual function of semiconductor nanocrystals |
| topic_facet |
CdTe nanocrystals Dual function Dual role Efficiency of energy transfer Efficient energy transfer Energy-transfer rate Exciton diffusion Hybrid structure Layer-by-layers Non-radiative recombinations Organic/inorganic nano-composite Semiconductor nanocrystals Cadmium compounds Energy transfer Excitons Nanocomposites Nanocrystals Conjugated polymers |
| description |
The efficiency of energy transfer in hybrid organic/inorganic nanocomposites based on conjugated polymers and semiconductor nanocrystals is strongly dependent on both the energy transfer rate and the rate of the nonradiative recombination of the polymer. We demonstrate that the polymer nonradiative recombination can be reduced by the suppression of exciton diffusion via proper morphology engineering of a hybrid structure. In the layer-by-layer assembled nanocomposite of a conjugated polymer and CdTe nanocrystals the latter have a dual role: first, they are efficient exciton acceptors and, second, they reduce nonradiative recombination in the polymer by suppressing exciton diffusion across the layers. © 2010 American Institute of Physics. |
| format |
JOUR |
| author |
Lutich, A.A. Pöschl, A. Jiang, G. Stefani, F.D. Susha, A.S. Rogach, A.L. Feldmann, J. |
| author_facet |
Lutich, A.A. Pöschl, A. Jiang, G. Stefani, F.D. Susha, A.S. Rogach, A.L. Feldmann, J. |
| author_sort |
Lutich, A.A. |
| title |
Efficient energy transfer in layered hybrid organic/inorganic nanocomposites: A dual function of semiconductor nanocrystals |
| title_short |
Efficient energy transfer in layered hybrid organic/inorganic nanocomposites: A dual function of semiconductor nanocrystals |
| title_full |
Efficient energy transfer in layered hybrid organic/inorganic nanocomposites: A dual function of semiconductor nanocrystals |
| title_fullStr |
Efficient energy transfer in layered hybrid organic/inorganic nanocomposites: A dual function of semiconductor nanocrystals |
| title_full_unstemmed |
Efficient energy transfer in layered hybrid organic/inorganic nanocomposites: A dual function of semiconductor nanocrystals |
| title_sort |
efficient energy transfer in layered hybrid organic/inorganic nanocomposites: a dual function of semiconductor nanocrystals |
| url |
http://hdl.handle.net/20.500.12110/paper_00036951_v96_n8_p_Lutich |
| work_keys_str_mv |
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| _version_ |
1807322625672740864 |