Hierarchical ZnO nanostructures: Growth mechanisms and surface correlated photoluminescence
ZnO nanowires were grown by vapor-transport and deposition on Au nanocluster covered fused and thermal silica and c-Si. The nanowire size and density depended strongly on the substrate type. By decreasing the O 2 to local Zn partial pressure ratio, the growth pattern changed to nanocombs and nanoshe...
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todo:paper_00036951_v100_n23_p_Grinblat2023-10-03T13:56:32Z Hierarchical ZnO nanostructures: Growth mechanisms and surface correlated photoluminescence Grinblat, G. Capeluto, M.G. Tirado, M. Bragas, A.V. Comedi, D. Au nanoclusters Exciton photoluminescences Growth mechanisms Growth patterns Morphology changes Nanocombs Partial pressure ratio Substrate types Two-dimensional growth ZnO ZnO nanostructures ZnO nanowires Fused silica Nanowires Photoluminescence Silicon Vapors Zinc oxide ZnO nanowires were grown by vapor-transport and deposition on Au nanocluster covered fused and thermal silica and c-Si. The nanowire size and density depended strongly on the substrate type. By decreasing the O 2 to local Zn partial pressure ratio, the growth pattern changed to nanocombs and nanosheets. ZnO nanohedgehogs were found on bare c-Si. We observe a remarkable correlation between the defect to exciton photoluminescence intensity ratio and the nanostructures specific surface areas. These results indicate that changes in strain and O deficiency defects at surfaces are behind the observed morphology changes, one to two-dimensional growth transition, and corresponding luminescence. © 2012 American Institute of Physics. JOUR info:eu-repo/semantics/openAccess http://creativecommons.org/licenses/by/2.5/ar http://hdl.handle.net/20.500.12110/paper_00036951_v100_n23_p_Grinblat |
institution |
Universidad de Buenos Aires |
institution_str |
I-28 |
repository_str |
R-134 |
collection |
Biblioteca Digital - Facultad de Ciencias Exactas y Naturales (UBA) |
topic |
Au nanoclusters Exciton photoluminescences Growth mechanisms Growth patterns Morphology changes Nanocombs Partial pressure ratio Substrate types Two-dimensional growth ZnO ZnO nanostructures ZnO nanowires Fused silica Nanowires Photoluminescence Silicon Vapors Zinc oxide |
spellingShingle |
Au nanoclusters Exciton photoluminescences Growth mechanisms Growth patterns Morphology changes Nanocombs Partial pressure ratio Substrate types Two-dimensional growth ZnO ZnO nanostructures ZnO nanowires Fused silica Nanowires Photoluminescence Silicon Vapors Zinc oxide Grinblat, G. Capeluto, M.G. Tirado, M. Bragas, A.V. Comedi, D. Hierarchical ZnO nanostructures: Growth mechanisms and surface correlated photoluminescence |
topic_facet |
Au nanoclusters Exciton photoluminescences Growth mechanisms Growth patterns Morphology changes Nanocombs Partial pressure ratio Substrate types Two-dimensional growth ZnO ZnO nanostructures ZnO nanowires Fused silica Nanowires Photoluminescence Silicon Vapors Zinc oxide |
description |
ZnO nanowires were grown by vapor-transport and deposition on Au nanocluster covered fused and thermal silica and c-Si. The nanowire size and density depended strongly on the substrate type. By decreasing the O 2 to local Zn partial pressure ratio, the growth pattern changed to nanocombs and nanosheets. ZnO nanohedgehogs were found on bare c-Si. We observe a remarkable correlation between the defect to exciton photoluminescence intensity ratio and the nanostructures specific surface areas. These results indicate that changes in strain and O deficiency defects at surfaces are behind the observed morphology changes, one to two-dimensional growth transition, and corresponding luminescence. © 2012 American Institute of Physics. |
format |
JOUR |
author |
Grinblat, G. Capeluto, M.G. Tirado, M. Bragas, A.V. Comedi, D. |
author_facet |
Grinblat, G. Capeluto, M.G. Tirado, M. Bragas, A.V. Comedi, D. |
author_sort |
Grinblat, G. |
title |
Hierarchical ZnO nanostructures: Growth mechanisms and surface correlated photoluminescence |
title_short |
Hierarchical ZnO nanostructures: Growth mechanisms and surface correlated photoluminescence |
title_full |
Hierarchical ZnO nanostructures: Growth mechanisms and surface correlated photoluminescence |
title_fullStr |
Hierarchical ZnO nanostructures: Growth mechanisms and surface correlated photoluminescence |
title_full_unstemmed |
Hierarchical ZnO nanostructures: Growth mechanisms and surface correlated photoluminescence |
title_sort |
hierarchical zno nanostructures: growth mechanisms and surface correlated photoluminescence |
url |
http://hdl.handle.net/20.500.12110/paper_00036951_v100_n23_p_Grinblat |
work_keys_str_mv |
AT grinblatg hierarchicalznonanostructuresgrowthmechanismsandsurfacecorrelatedphotoluminescence AT capelutomg hierarchicalznonanostructuresgrowthmechanismsandsurfacecorrelatedphotoluminescence AT tiradom hierarchicalznonanostructuresgrowthmechanismsandsurfacecorrelatedphotoluminescence AT bragasav hierarchicalznonanostructuresgrowthmechanismsandsurfacecorrelatedphotoluminescence AT comedid hierarchicalznonanostructuresgrowthmechanismsandsurfacecorrelatedphotoluminescence |
_version_ |
1807316054514335744 |