A nonlinear switching mechanism in quantum dot and metallic nanoparticle hybrid systems
Second harmonic generation and two-photon photoluminescence in CdS quantum dots near metallic nanoparticles are theoretically and experimentally investigated. A control laser field is applied to the hybrid system, which couples with the surface plasmons of the metal nanoparticles. The polarized meta...
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Acceso en línea: | https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_21951071_v1_n6_p460_Cox http://hdl.handle.net/20.500.12110/paper_21951071_v1_n6_p460_Cox |
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paper:paper_21951071_v1_n6_p460_Cox2023-06-08T16:35:08Z A nonlinear switching mechanism in quantum dot and metallic nanoparticle hybrid systems von Bilderling, Catalina Bragas, Andrea Verónica Hybrid nanomaterials Metallic nanoparticles Quantum dots Second harmonic generation Switching mechanisms Second harmonic generation and two-photon photoluminescence in CdS quantum dots near metallic nanoparticles are theoretically and experimentally investigated. A control laser field is applied to the hybrid system, which couples with the surface plasmons of the metal nanoparticles. The polarized metal nanoparticles then interact with the quantum dots through dipole-dipole interactions, which enhances the intensity of the second harmonic signal from the quantum dots. The density matrix method is used to numerically simulate the second harmonic signal emitted by the quantum dots. It is found that the enhancement of the second harmonic signal can be switched on and off by changing the control field intensity. Alternatively, the second harmonic signal enhancement can be turned on or off by changing the frequency of the control field. This is an interesting finding which can be used to fabricate nonlinear all optical nanoswitching devices from hybrid systems. © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. Fil:von Bilderling, C. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales; Argentina. Fil:Bragas, A.V. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales; Argentina. 2013 https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_21951071_v1_n6_p460_Cox http://hdl.handle.net/20.500.12110/paper_21951071_v1_n6_p460_Cox |
institution |
Universidad de Buenos Aires |
institution_str |
I-28 |
repository_str |
R-134 |
collection |
Biblioteca Digital - Facultad de Ciencias Exactas y Naturales (UBA) |
topic |
Hybrid nanomaterials Metallic nanoparticles Quantum dots Second harmonic generation Switching mechanisms |
spellingShingle |
Hybrid nanomaterials Metallic nanoparticles Quantum dots Second harmonic generation Switching mechanisms von Bilderling, Catalina Bragas, Andrea Verónica A nonlinear switching mechanism in quantum dot and metallic nanoparticle hybrid systems |
topic_facet |
Hybrid nanomaterials Metallic nanoparticles Quantum dots Second harmonic generation Switching mechanisms |
description |
Second harmonic generation and two-photon photoluminescence in CdS quantum dots near metallic nanoparticles are theoretically and experimentally investigated. A control laser field is applied to the hybrid system, which couples with the surface plasmons of the metal nanoparticles. The polarized metal nanoparticles then interact with the quantum dots through dipole-dipole interactions, which enhances the intensity of the second harmonic signal from the quantum dots. The density matrix method is used to numerically simulate the second harmonic signal emitted by the quantum dots. It is found that the enhancement of the second harmonic signal can be switched on and off by changing the control field intensity. Alternatively, the second harmonic signal enhancement can be turned on or off by changing the frequency of the control field. This is an interesting finding which can be used to fabricate nonlinear all optical nanoswitching devices from hybrid systems. © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. |
author |
von Bilderling, Catalina Bragas, Andrea Verónica |
author_facet |
von Bilderling, Catalina Bragas, Andrea Verónica |
author_sort |
von Bilderling, Catalina |
title |
A nonlinear switching mechanism in quantum dot and metallic nanoparticle hybrid systems |
title_short |
A nonlinear switching mechanism in quantum dot and metallic nanoparticle hybrid systems |
title_full |
A nonlinear switching mechanism in quantum dot and metallic nanoparticle hybrid systems |
title_fullStr |
A nonlinear switching mechanism in quantum dot and metallic nanoparticle hybrid systems |
title_full_unstemmed |
A nonlinear switching mechanism in quantum dot and metallic nanoparticle hybrid systems |
title_sort |
nonlinear switching mechanism in quantum dot and metallic nanoparticle hybrid systems |
publishDate |
2013 |
url |
https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_21951071_v1_n6_p460_Cox http://hdl.handle.net/20.500.12110/paper_21951071_v1_n6_p460_Cox |
work_keys_str_mv |
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_version_ |
1768546744433377280 |