Non-plasmonic nanoantennas for surface enhanced spectroscopies with ultra-low heat conversion

Nanoplasmonics has recently revolutionized our ability to control light on the nanoscale. Using metallic nanostructures with tailored shapes, it is possible to efficiently focus light into nanoscale field 'hot spots'. High field enhancement factors have been achieved in such optical nanoan...

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Autor principal: Bragas, Andrea Verónica
Publicado: 2015
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Acceso en línea:https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_20411723_v6_n_p_Caldarola
http://hdl.handle.net/20.500.12110/paper_20411723_v6_n_p_Caldarola
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spelling paper:paper_20411723_v6_n_p_Caldarola2023-06-08T16:33:07Z Non-plasmonic nanoantennas for surface enhanced spectroscopies with ultra-low heat conversion Bragas, Andrea Verónica dimer gold nanomaterial silicon fluorescence heat balance light effect molecular analysis nonlinearity optical property Raman spectroscopy silicon spectroscopy temperature effect Article electromagnetic field fluorescence heating molecular electronics nanofabrication Raman spectrometry spectroscopy temperature Nanoplasmonics has recently revolutionized our ability to control light on the nanoscale. Using metallic nanostructures with tailored shapes, it is possible to efficiently focus light into nanoscale field 'hot spots'. High field enhancement factors have been achieved in such optical nanoantennas, enabling transformative science in the areas of single molecule interactions, highly enhanced nonlinearities and nanoscale waveguiding. Unfortunately, these large enhancements come at the price of high optical losses due to absorption in the metal, severely limiting real-world applications. Via the realization of a novel nanophotonic platform based on dielectric nanostructures to form efficient nanoantennas with ultra-low light-into-heat conversion, here we demonstrate an approach that overcomes these limitations. We show that dimer-like silicon-based single nanoantennas produce both high surface enhanced fluorescence and surface enhanced Raman scattering, while at the same time generating a negligible temperature increase in their hot spots and surrounding environments. © 2015 Macmillan Publishers Limited. All rights reserved. Fil:Bragas, A.V. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales; Argentina. 2015 https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_20411723_v6_n_p_Caldarola http://hdl.handle.net/20.500.12110/paper_20411723_v6_n_p_Caldarola
institution Universidad de Buenos Aires
institution_str I-28
repository_str R-134
collection Biblioteca Digital - Facultad de Ciencias Exactas y Naturales (UBA)
topic dimer
gold
nanomaterial
silicon
fluorescence
heat balance
light effect
molecular analysis
nonlinearity
optical property
Raman spectroscopy
silicon
spectroscopy
temperature effect
Article
electromagnetic field
fluorescence
heating
molecular electronics
nanofabrication
Raman spectrometry
spectroscopy
temperature
spellingShingle dimer
gold
nanomaterial
silicon
fluorescence
heat balance
light effect
molecular analysis
nonlinearity
optical property
Raman spectroscopy
silicon
spectroscopy
temperature effect
Article
electromagnetic field
fluorescence
heating
molecular electronics
nanofabrication
Raman spectrometry
spectroscopy
temperature
Bragas, Andrea Verónica
Non-plasmonic nanoantennas for surface enhanced spectroscopies with ultra-low heat conversion
topic_facet dimer
gold
nanomaterial
silicon
fluorescence
heat balance
light effect
molecular analysis
nonlinearity
optical property
Raman spectroscopy
silicon
spectroscopy
temperature effect
Article
electromagnetic field
fluorescence
heating
molecular electronics
nanofabrication
Raman spectrometry
spectroscopy
temperature
description Nanoplasmonics has recently revolutionized our ability to control light on the nanoscale. Using metallic nanostructures with tailored shapes, it is possible to efficiently focus light into nanoscale field 'hot spots'. High field enhancement factors have been achieved in such optical nanoantennas, enabling transformative science in the areas of single molecule interactions, highly enhanced nonlinearities and nanoscale waveguiding. Unfortunately, these large enhancements come at the price of high optical losses due to absorption in the metal, severely limiting real-world applications. Via the realization of a novel nanophotonic platform based on dielectric nanostructures to form efficient nanoantennas with ultra-low light-into-heat conversion, here we demonstrate an approach that overcomes these limitations. We show that dimer-like silicon-based single nanoantennas produce both high surface enhanced fluorescence and surface enhanced Raman scattering, while at the same time generating a negligible temperature increase in their hot spots and surrounding environments. © 2015 Macmillan Publishers Limited. All rights reserved.
author Bragas, Andrea Verónica
author_facet Bragas, Andrea Verónica
author_sort Bragas, Andrea Verónica
title Non-plasmonic nanoantennas for surface enhanced spectroscopies with ultra-low heat conversion
title_short Non-plasmonic nanoantennas for surface enhanced spectroscopies with ultra-low heat conversion
title_full Non-plasmonic nanoantennas for surface enhanced spectroscopies with ultra-low heat conversion
title_fullStr Non-plasmonic nanoantennas for surface enhanced spectroscopies with ultra-low heat conversion
title_full_unstemmed Non-plasmonic nanoantennas for surface enhanced spectroscopies with ultra-low heat conversion
title_sort non-plasmonic nanoantennas for surface enhanced spectroscopies with ultra-low heat conversion
publishDate 2015
url https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_20411723_v6_n_p_Caldarola
http://hdl.handle.net/20.500.12110/paper_20411723_v6_n_p_Caldarola
work_keys_str_mv AT bragasandreaveronica nonplasmonicnanoantennasforsurfaceenhancedspectroscopieswithultralowheatconversion
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