Instability scenarios for doped 4He clusters
In the frame of finite range density functional (FRDF) theory, we review the systematics of energetic features of 4HeN clusters doped with atomic or molecular impurities, as well as the instability scenario of their collective motions. It is shown that for drops up to N = 500, the predictions of FRD...
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1997
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Acceso en línea: | http://hdl.handle.net/20.500.12110/paper_00219606_v107_n3_p927_Gatica http://repositoriouba.sisbi.uba.ar/gsdl/cgi-bin/library.cgi?a=d&c=artiaex&d=paper_00219606_v107_n3_p927_Gatica_oai |
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I28-R145-paper_00219606_v107_n3_p927_Gatica_oai2020-10-19 Gatica, S.M. Hernández, E.S. Barranco, M. 1997 In the frame of finite range density functional (FRDF) theory, we review the systematics of energetic features of 4HeN clusters doped with atomic or molecular impurities, as well as the instability scenario of their collective motions. It is shown that for drops up to N = 500, the predictions of FRDF theory are coincident with those arising from microscopic many-body calculations that employ variational or diffusion Monte Carlo methods. For larger drops, the present description predicts a smooth approach to zero of the collective energies, a scenario that appears to support the most recent experimental data and microscopic calculations that demonstrate that the impurity is located within the bulk of the drop. © 1997 American Institute of Physics. Fil:Gatica, S.M. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales; Argentina. Fil:Hernández, E.S. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales; Argentina. application/pdf http://hdl.handle.net/20.500.12110/paper_00219606_v107_n3_p927_Gatica info:eu-repo/semantics/openAccess http://creativecommons.org/licenses/by/2.5/ar J Chem Phys 1997;107(3):927-931 Instability scenarios for doped 4He clusters info:eu-repo/semantics/article info:ar-repo/semantics/artículo info:eu-repo/semantics/publishedVersion http://repositoriouba.sisbi.uba.ar/gsdl/cgi-bin/library.cgi?a=d&c=artiaex&d=paper_00219606_v107_n3_p927_Gatica_oai |
institution |
Universidad de Buenos Aires |
institution_str |
I-28 |
repository_str |
R-145 |
collection |
Repositorio Digital de la Universidad de Buenos Aires (UBA) |
description |
In the frame of finite range density functional (FRDF) theory, we review the systematics of energetic features of 4HeN clusters doped with atomic or molecular impurities, as well as the instability scenario of their collective motions. It is shown that for drops up to N = 500, the predictions of FRDF theory are coincident with those arising from microscopic many-body calculations that employ variational or diffusion Monte Carlo methods. For larger drops, the present description predicts a smooth approach to zero of the collective energies, a scenario that appears to support the most recent experimental data and microscopic calculations that demonstrate that the impurity is located within the bulk of the drop. © 1997 American Institute of Physics. |
format |
Artículo Artículo publishedVersion |
author |
Gatica, S.M. Hernández, E.S. Barranco, M. |
spellingShingle |
Gatica, S.M. Hernández, E.S. Barranco, M. Instability scenarios for doped 4He clusters |
author_facet |
Gatica, S.M. Hernández, E.S. Barranco, M. |
author_sort |
Gatica, S.M. |
title |
Instability scenarios for doped 4He clusters |
title_short |
Instability scenarios for doped 4He clusters |
title_full |
Instability scenarios for doped 4He clusters |
title_fullStr |
Instability scenarios for doped 4He clusters |
title_full_unstemmed |
Instability scenarios for doped 4He clusters |
title_sort |
instability scenarios for doped 4he clusters |
publishDate |
1997 |
url |
http://hdl.handle.net/20.500.12110/paper_00219606_v107_n3_p927_Gatica http://repositoriouba.sisbi.uba.ar/gsdl/cgi-bin/library.cgi?a=d&c=artiaex&d=paper_00219606_v107_n3_p927_Gatica_oai |
work_keys_str_mv |
AT gaticasm instabilityscenariosfordoped4heclusters AT hernandezes instabilityscenariosfordoped4heclusters AT barrancom instabilityscenariosfordoped4heclusters |
_version_ |
1766026562824568832 |