Identification of essential amino acids in the bacterial α-mannosyltransferase AceA

The α-mannosyltransferase AceA from Acetobacter xylinum belongs to the CaZY family 4 of retaining glycosyltransferases. We have identified a series of either highly conserved or invariant residues that are found in all family 4 enzymes as well as other retaining glycosyltransferases. These residues...

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Autor principal: Abdian, P.L
Otros Autores: Lellouch, A.C, Gautier, C., Ielpi, L., Geremia, R.A
Formato: Capítulo de libro
Lenguaje:Inglés
Publicado: 2000
Acceso en línea:Registro en Scopus
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024 7 |2 scopus  |a 2-s2.0-0034704103 
024 7 |2 cas  |a Amino Acids, Essential; GDP-mannose - cellobiosyl-diphosphopolyprenol mannosyltransferase, EC 2.4.1.-; Mannosyltransferases, EC 2.4.1.-; Recombinant Proteins 
040 |a Scopus  |b spa  |c AR-BaUEN  |d AR-BaUEN 
030 |a JBCHA 
100 1 |a Abdian, P.L. 
245 1 0 |a Identification of essential amino acids in the bacterial α-mannosyltransferase AceA 
260 |c 2000 
270 1 0 |m Geremia, R.A.; CERMAV/CNRS, BP 53, 38041 Grenoble Cedex 9, France; email: roberto.geremia@cermav.cnrs.fr 
506 |2 openaire  |e Política editorial 
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504 |a Geremia, R.A., Petroni, E.A., Ielpi, L., Henrissat, B., (1996) Biochem. J., 318, pp. 133-1338 
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504 |a Filisetti-Cozzi, T.M., Carpita, N.C., (1991) Anal. Biochem., 197, pp. 157-162 
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504 |a Cid, E., Gomis, R.R., Geremia, R.A., Guinovart, J.J., Ferrer, J.C., (2000) J. Biol. Chem., 275, pp. 33614-33621 
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520 3 |a The α-mannosyltransferase AceA from Acetobacter xylinum belongs to the CaZY family 4 of retaining glycosyltransferases. We have identified a series of either highly conserved or invariant residues that are found in all family 4 enzymes as well as other retaining glycosyltransferases. These residues included Glu-287 and Glu-295, which comprise an EX7E motif and have been proposed to be involved in catalysis. Alanine replacements of each conserved residue were constructed by site-directed mutagenesis. The mannosyltransferase activity of each mutant was examined by both an in vitro transferase assay using recombinant mutant AceA expressed in Escherichia coli and by an in vivo rescue assay by expressing the mutant AceA in a Xanthomonas campestris gumH- strain. We found that only mutants K211A and E287A lost all detectable activity both in vitro and in vivo, whereas E295A retained residual activity in the more sensitive in vivo assay. H127A and S162A each retained reduced but significant activities both in vitro and in vivo. Secondary structure predictions of AceA and subsequent comparison with the crystal structures of the T4 β-glucosyltransferase and MurG suggest that AceA Lys-211 and Glu-295 are involved in nucleotide sugar donor binding, leaving Glu-287 of the EX7E as a potential catalytic residue.  |l eng 
593 |a Instituto de Investigaciones Bioquímicas Fundación Campomar, Facultad de Ciencias Exactas y Naturales, Consejo Nacional de Investigaciones Científicas y Técnicas, Avenida Patricias Argentinas 435, 1045 Buenos Aires, Argentina 
593 |a Centre de Recherches Sur Les Macromolécules Végétales, CNRS, Joseph Fourier University, BP 53X, 38041 Grenoble Cedex 9, France 
593 |a CERMAV/CNRS, BP 53, 38041 Grenoble Cedex 9, France 
593 |a Carrera del Investigador, Consejo Nacional de Investigaciones CientIficas y Técnicas, Buenos Aires, Argentina 
690 1 0 |a ALPHA MANNOSYLTRANSFERASE ACEA 
690 1 0 |a BACTERIAL ENZYME 
690 1 0 |a ESSENTIAL AMINO ACID 
690 1 0 |a GLUCOSYLTRANSFERASE 
690 1 0 |a MANNOSYLTRANSFERASE 
690 1 0 |a UNCLASSIFIED DRUG 
690 1 0 |a ACETOBACTER 
690 1 0 |a AMINO ACID SUBSTITUTION 
690 1 0 |a ARTICLE 
690 1 0 |a CELLULAR DISTRIBUTION 
690 1 0 |a ENZYME ACTIVITY 
690 1 0 |a ENZYME ANALYSIS 
690 1 0 |a ENZYME STRUCTURE 
690 1 0 |a NONHUMAN 
690 1 0 |a PRIORITY JOURNAL 
690 1 0 |a STRUCTURE ANALYSIS 
690 1 0 |a ACETOBACTER 
690 1 0 |a AMINO ACIDS, ESSENTIAL 
690 1 0 |a CATALYSIS 
690 1 0 |a MANNOSYLTRANSFERASES 
690 1 0 |a NUCLEAR MAGNETIC RESONANCE, BIOMOLECULAR 
690 1 0 |a PROTEIN STRUCTURE, SECONDARY 
690 1 0 |a RECOMBINANT PROTEINS 
690 1 0 |a ACETOBACTER 
690 1 0 |a BACTERIA (MICROORGANISMS) 
690 1 0 |a ESCHERICHIA COLI 
690 1 0 |a GLUCONACETOBACTER XYLINUS 
690 1 0 |a XANTHOMONAS CAMPESTRIS 
700 1 |a Lellouch, A.C. 
700 1 |a Gautier, C. 
700 1 |a Ielpi, L. 
700 1 |a Geremia, R.A. 
773 0 |d 2000  |g v. 275  |h pp. 40568-40575  |k n. 51  |p J. Biol. Chem.  |x 00219258  |w (AR-BaUEN)CENRE-175  |t Journal of Biological Chemistry 
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856 4 0 |u https://doi.org/10.1074/jbc.M007496200  |y DOI 
856 4 0 |u https://hdl.handle.net/20.500.12110/paper_00219258_v275_n51_p40568_Abdian  |y Handle 
856 4 0 |u https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_00219258_v275_n51_p40568_Abdian  |y Registro en la Biblioteca Digital 
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963 |a NORI 
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