Mixed-valent diruthenium (II,III) aliphatic carboxylates: Columnar mesophases in dodecylsulfate and octylsulfonate derivatives

Two series of polymeric mixed-valent diruthenium (II,III) aliphatic carboxylates of formula Ru2[O2C(CH2) n-2CH3]4X (where X=dodecylsulfate (DOS) anion and n=8, 9, 16 and 18, or X=octylsulfonate (OS) anion and n=8, 10, 12, 14 and 18) were synthesized and characterized. Their liquid crystalline proper...

Descripción completa

Guardado en:
Detalles Bibliográficos
Autor principal: Chaia, Z.
Otros Autores: Zelcer, A., Donnio, B., Rusjan, M., Cukiernik, F.D, Guillon, D.
Formato: Capítulo de libro
Lenguaje:Inglés
Publicado: 2004
Acceso en línea:Registro en Scopus
DOI
Handle
Registro en la Biblioteca Digital
Aporte de:Registro referencial: Solicitar el recurso aquí
LEADER 05198caa a22007097a 4500
001 PAPER-21216
003 AR-BaUEN
005 20230518205239.0
008 190411s2004 xx ||||fo|||| 00| 0 eng|d
024 7 |2 scopus  |a 2-s2.0-3242687160 
024 7 |2 cas  |a dodecyl sulfate, 151-41-7; octane, 111-65-9; ruthenium, 7440-18-8 
040 |a Scopus  |b spa  |c AR-BaUEN  |d AR-BaUEN 
030 |a LICRE 
100 1 |a Chaia, Z. 
245 1 0 |a Mixed-valent diruthenium (II,III) aliphatic carboxylates: Columnar mesophases in dodecylsulfate and octylsulfonate derivatives 
260 |c 2004 
270 1 0 |m Cukiernik, F.D.; INQUIMAE, Departamento de Quimica Inorganica, Universidad de Buenos Aires, C1428EHA Buenos Aires, Argentina; email: fcukiern@ungs.edu.ar 
506 |2 openaire  |e Política editorial 
504 |a Aquino, M.A.S., (1998) Coord. Chem. Rev., 170, p. 141 
504 |a Cukiernik, F.D., Maldivi, P., Giroud-Godquin, A.M., Marchon, J.C., Ibn-Elhaj, M., Guillon, D., Skoulios, A., (1991) Liq. Cryst., 9, p. 903 
504 |a Cukiernik, F.D., Ibn-Elhaj, M., Chaia, Z., Marchon, J.C., Giroud-Godquin, A.M., Guillon, D., Skoulios, A., Maldivi, P., (1998) Chem. Mater., 10, p. 83 
504 |a Chaia, Z., Heinrich, B., Cukiernik, F.D., Guillon, D., (1999) Mol. Cryst. Liq. Cryst., 330, p. 213 
504 |a Guillon, D., (1999) Struct. Bonding (Berlin), 95, p. 42 
504 |a Caplan, J.F., Murphy, C.A., Swansburg, S., Lemieux, R.P., Cameron, T.S., Aquino, M.A.S., (1998) Can. J. Chem., 76, p. 1520 
504 |a Zelcer, A., Chaia, Z., Cukiernik, F.D., Castellano, E.E., Piro, O.E., (2002) Acta Cryst., C58, pp. m144 
504 |a Nakamoto, K., (1986) Infrared and Raman Spectra of Inorganic and Coordination Compounds, 4th Edn, , New York: John Wiley 
504 |a Guillon, D., Skoulios, A., Benattar, J.J., (1986) J. Phys., 47, p. 133 
520 3 |a Two series of polymeric mixed-valent diruthenium (II,III) aliphatic carboxylates of formula Ru2[O2C(CH2) n-2CH3]4X (where X=dodecylsulfate (DOS) anion and n=8, 9, 16 and 18, or X=octylsulfonate (OS) anion and n=8, 10, 12, 14 and 18) were synthesized and characterized. Their liquid crystalline properties and crystalline (Cr) structures were analysed; the Cr phases are lamellar in all cases. For long chain DOS derivatives (n=16 and 18) hexagonal and rectangular columnar mesophases (Colh and Colr) with melting temperatures close to 140°C were observed. For long chain OS derivatives (n ≥ 10) a Colh mesophase was observed, with melting temperatures between 140 and 190°C.  |l eng 
536 |a Detalles de la financiación: Universidad de Buenos Aires, EX117, AX27 
536 |a Detalles de la financiación: Fundación Antorchas 
536 |a Detalles de la financiación: Agencia Nacional de Promoción Científica y Tecnológica, 546, PEI 121/98, A97E08 
536 |a Detalles de la financiación: We wish to thank Drs P. Maldivi and J.C. Marchon (CEA/Grenoble) for help at the beginning of this work, as well as B. Heinrich (GMO-IPCMS) for help during the X-ray diffraction investigations. Financial Support from the University of Buenos Aires (EX117 and AX27), Fundación Antorchas, ANPCyT (546), Conicet (PEI 121/98) and Ecos-Secyt (grant A97E08 for international cooperation) is acknowledged. Z.D.C. and M.R. thank CONICET for doctoral fellowships. A.Z. thanks UBA for a student fellowship. F.D.C. is a member of the scientific staff of CONICET. 
593 |a INQUIMAE, Departamento de Quimica Inorganica, Universidad de Buenos Aires, C1428EHA Buenos Aires, Argentina 
593 |a Inst. Phys./Chim. Mat. de Strasbourg, Grp. des Mat. Organiques (GMO-IPCMS), 23 Rue de Loess, 67034 Strasbourg Cedex 2, France 
593 |a Instituto de Ciencias, Univ. Nacional de General Sarmiento, J. M. Gutierrez 1150, Los Polvorines, Prov. Buenos Aires, Argentina 
690 1 0 |a ALIPHATIC COMPOUND 
690 1 0 |a CARBOXYLIC ACID DERIVATIVE 
690 1 0 |a DODECYL SULFATE 
690 1 0 |a OCTANE 
690 1 0 |a POLYMER 
690 1 0 |a RUTHENIUM 
690 1 0 |a SULFONIC ACID DERIVATIVE 
690 1 0 |a ARTICLE 
690 1 0 |a CRYSTAL STRUCTURE 
690 1 0 |a LIQUID CRYSTAL 
690 1 0 |a MELTING POINT 
690 1 0 |a MESOPHASE 
690 1 0 |a PHYSICAL CHEMISTRY 
690 1 0 |a SYNTHESIS 
700 1 |a Zelcer, A. 
700 1 |a Donnio, B. 
700 1 |a Rusjan, M. 
700 1 |a Cukiernik, F.D. 
700 1 |a Guillon, D. 
773 0 |d 2004  |g v. 31  |h pp. 1019-1025  |k n. 7  |p Liq. Cryst.  |x 02678292  |w (AR-BaUEN)CENRE-5971  |t Liquid Crystals 
856 4 1 |u https://www.scopus.com/inward/record.uri?eid=2-s2.0-3242687160&doi=10.1080%2f02678290410001713333&partnerID=40&md5=1381e4d4577e1121b7c526c468ac81ab  |y Registro en Scopus 
856 4 0 |u https://doi.org/10.1080/02678290410001713333  |y DOI 
856 4 0 |u https://hdl.handle.net/20.500.12110/paper_02678292_v31_n7_p1019_Chaia  |y Handle 
856 4 0 |u https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_02678292_v31_n7_p1019_Chaia  |y Registro en la Biblioteca Digital 
961 |a paper_02678292_v31_n7_p1019_Chaia  |b paper  |c PE 
962 |a info:eu-repo/semantics/article  |a info:ar-repo/semantics/artículo  |b info:eu-repo/semantics/publishedVersion 
999 |c 82169