CeIV–GdIII Mixed Oxides as Hosts for ErIII-Based Upconversion Phosphors

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A family of ErIII and ErIII–YbIII based nanophosphors, hosted in monophasic oxidic CeIV–GdIII binary solid solutions, was prepared. The samples were formulated with a constant ErIII content as the activator, with the eventual addition of YbIII as a sensitizer. The amorphous Ce0.94−xGdxEr0.06(OH)CO3H...

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Autor principal: Sorbello, C.
Otros Autores: Gross, P., Strassert, C.A, Jobbágy, M., Barja, B.C
Formato: Capítulo de libro
Lenguaje:Inglés
Publicado: Wiley-VCH Verlag 2017
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Biblioteca Central Dr. Luis F. Leloir (FCEN) de Universidad de Buenos Aires
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100 1 |a Sorbello, C. 
245 1 0 |a CeIV–GdIII Mixed Oxides as Hosts for ErIII-Based Upconversion Phosphors 
260 |b Wiley-VCH Verlag  |c 2017 
270 1 0 |m Jobbágy, M.; Departamento de Química Inorgánica Analítica y Química Física FCEyN-Universidad de Buenos Aires, INQUIMAE-CONICET, CABA, Ciudad Universitaria Pabellón 2, Argentina; email: jobbag@qi.fcen.uba.ar 
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520 3 |a A family of ErIII and ErIII–YbIII based nanophosphors, hosted in monophasic oxidic CeIV–GdIII binary solid solutions, was prepared. The samples were formulated with a constant ErIII content as the activator, with the eventual addition of YbIII as a sensitizer. The amorphous Ce0.94−xGdxEr0.06(OH)CO3H2O and Ce0.94−xGdxEr0.05Yb0.01(OH)CO3H2O precursors were prepared by following the urea method to obtain monodispersed spheres of tunable size ranging from 30 to 450 nm. After being decomposed at 1273 K under an atmosphere of air, the precursors of 200 nm in diameter evolved into monophasic polycrystalline particles preserving the parent shape and size. The role of the composition of the binary matrices in the emission properties was evaluated for two different excitation wavelengths (976 nm and 780 nm) based on the upconversion (UC) emission spectra and their dependence on the incident power. The yield of the UC process is discussed in the framework of established and novel alternative mechanisms. The number of vacancies and mainly the symmetry of the ErIII environment play major roles in the deactivation pathways of the UC emission mechanisms. However, the colours obtained by employing bare CeIV or GdIII hosts are preserved in the related monophasic CeIV-rich or GdIII-rich binary hosts. © 2017 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim  |l eng 
536 |a Detalles de la financiación: PIP 11220110101020 
536 |a Detalles de la financiación: Universidad de Buenos Aires, UBACyT 20020130100610BA 
536 |a Detalles de la financiación: Consejo Nacional de Investigaciones Científicas y Técnicas 
536 |a Detalles de la financiación: Deutscher Akademischer Austausch Dienst Kairo 
536 |a Detalles de la financiación: US-Egypt Joint Board on Scientific and Technological Cooperation 
536 |a Detalles de la financiación: Agencia Nacional de Promoción Científica y Tecnológica, PICT 2012-1167 
536 |a Detalles de la financiación: This work was supported by the University of Buenos Aires (UBACyT 20020130100610BA), the Agencia Nacional de Promoci?n Cient?fica y Tecnol?gica (ANPCyT PICT 2012-1167) and Consejo Nacional de Investigaciones Cient?ficas y T?cnicas (CONICET PIP 11220110101020). C.S. acknowledges CONICET for a doctoral fellowship. B.B. and M.J. are Research Scientist of CONICET (Argentina). B.C.B. thanks to the Deutscher Akademischer Austausch Dienst (DAAD) for the financial support received for an international research exchange within the Scientific and Technological Cooperation Program (Argentine-Germany). 
593 |a Departamento de Química Inorgánica Analítica y Química Física FCEyN-Universidad de Buenos Aires, INQUIMAE-CONICET, CABA, Ciudad Universitaria Pabellón 2C1428EHA, Argentina 
593 |a Institute for Physics, Carl von Ossietzky University, Carl-von-Ossietzky-Str. 9, Oldenburg, 26129, Germany 
593 |a Physikalisches Institut and Center for Nanotechnology (CeNTech), Westfälische Wilhelms-Universität Münster, Heisenbergstraße 11, Münster, 48149, Germany 
690 1 0 |a ENERGY TRANSFER 
690 1 0 |a LANTHANIDES 
690 1 0 |a LUMINESCENCE 
690 1 0 |a PHOTOCHEMISTRY 
690 1 0 |a SOLID-STATE STRUCTURES 
700 1 |a Gross, P. 
700 1 |a Strassert, C.A. 
700 1 |a Jobbágy, M. 
700 1 |a Barja, B.C. 
773 0 |d Wiley-VCH Verlag, 2017  |g v. 18  |h pp. 1407-1414  |k n. 10  |p ChemPhysChem  |x 14394235  |t ChemPhysChem 
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