Density modes in spherical 4He shells

We compute the density-fluctuation spectrum of spherical 4HeN shells adsorbed on the outer surface of C n fullerenes. The excitation spectrum is obtained within the random-phase approximation, with particle-hole elementary excitations and effective interaction extracted from a density-functional des...

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Autores principales: Barranco, M., Hernández, E.S., Mayol, R., Pi, M.
Formato: JOUR
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Acceso en línea:http://hdl.handle.net/20.500.12110/paper_01631829_v69_n13_p134502_Barranco
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Sumario:We compute the density-fluctuation spectrum of spherical 4HeN shells adsorbed on the outer surface of C n fullerenes. The excitation spectrum is obtained within the random-phase approximation, with particle-hole elementary excitations and effective interaction extracted from a density-functional description of the shell structure. The presence of one or two solid helium layers adjacent to the adsorbing fullerene is phenomenologically accounted for. We illustrate our results for a selection of numbers of adsorbed atoms on C20, C 60, and C120. The hydrodynamical model that has proven successful to describe helium excitations in the bulk and in restricted geometries permits to perform a rather exhaustive analysis of various fluid spherical systems, namely, spheres, cavities, free bubbles, and bound shells of variable size.