Quantum dots as templates for self-assembly of photoswitchable polymers: Small, dual-color nanoparticles capable of facile photomodulation

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A photomodulatable amphiphilic polymer has been synthesized with a backbone of poly[isobutylene-alt-maleic anhydride] and pendant dodecyl alkyl chains, Lucifer Yellow (LY) fluorescent probes, and diheteroarylethenes photochromic (PC) groups. The latter serve as reversible UV-activated FRET acceptors...

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Autor principal: Díaz, S.A
Otros Autores: Giordano, L., Azcárate, J.C, Jovin, T.M, Jares-Erijman, E.A
Formato: Capítulo de libro
Lenguaje:Inglés
Publicado: 2013
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Biblioteca Central Dr. Luis F. Leloir (FCEN) de Universidad de Buenos Aires
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100 1 |a Díaz, S.A. 
245 1 0 |a Quantum dots as templates for self-assembly of photoswitchable polymers: Small, dual-color nanoparticles capable of facile photomodulation 
260 |c 2013 
270 1 0 |m Jovin, T.M.; Laboratory of Cellular Dynamics, Max Planck Institute for Biophysical Chemistry, Am Fassberg 11, 37077 Göttingen, Germany; email: tjovin@gwdg.de 
506 |2 openaire  |e Política editorial 
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520 3 |a A photomodulatable amphiphilic polymer has been synthesized with a backbone of poly[isobutylene-alt-maleic anhydride] and pendant dodecyl alkyl chains, Lucifer Yellow (LY) fluorescent probes, and diheteroarylethenes photochromic (PC) groups. The latter serve as reversible UV-activated FRET acceptors for the LY donors. We characterized the spectral and switching properties of the polymer in an organic solvent (CHCl3). In an aqueous medium the polymer forms polymersomes, constituting fluorescence probes ∼75 nm in diameter. Self-assembly of the polymer on the surface of a quantum dot (QD) serving as a template creates a dual-color photoswitchable nanoparticle (psNP) with improved properties due to the increase in polymer density and efficiency of PC photoconversion. The psNP exhibits a second QD red emission band that functions as an internal standard requiring only a single excitation wavelength, and is much reduced in size (<20 nm diameter) compared to the polymersomes. The QD template also greatly increases the depth of modulation by photochromic FRET of the LY emission monitored by both steady-state and time-resolved (lifetime) fluorescence (from 20%→70%, and from 12%→55%, respectively). © 2013 American Chemical Society.  |l eng 
593 |a Laboratory of Cellular Dynamics, Max Planck Institute for Biophysical Chemistry, Am Fassberg 11, 37077 Göttingen, Germany 
593 |a Departamento de Química Orgánica, Facultad de Ciencias Exactas y Naturales, CONICET, 1428 Buenos Aires, Argentina 
593 |a Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas, Facultad de Ciencias Exactas, CONICET, La Plata, Argentina 
690 1 0 |a ALKYL CHAIN 
690 1 0 |a AMPHIPHILIC POLYMERS 
690 1 0 |a AQUEOUS MEDIUM 
690 1 0 |a DEPTH OF MODULATION 
690 1 0 |a DUAL COLOR 
690 1 0 |a FLUORESCENCE PROBES 
690 1 0 |a FLUORESCENT PROBES 
690 1 0 |a INTERNAL STANDARDS 
690 1 0 |a LUCIFER YELLOWS 
690 1 0 |a PHOTO MODULATION 
690 1 0 |a PHOTO-SWITCHABLE 
690 1 0 |a PHOTOCONVERSION 
690 1 0 |a POLYMER DENSITIES 
690 1 0 |a POLYMERSOMES 
690 1 0 |a RED EMISSION BAND 
690 1 0 |a SINGLE EXCITATION 
690 1 0 |a SWITCHING PROPERTIES 
690 1 0 |a TIME-RESOLVED 
690 1 0 |a BUTENES 
690 1 0 |a FLUORESCENCE 
690 1 0 |a MALEIC ANHYDRIDE 
690 1 0 |a NANOPARTICLES 
690 1 0 |a ORGANIC SOLVENTS 
690 1 0 |a PHOTOCHROMISM 
690 1 0 |a SELF ASSEMBLY 
690 1 0 |a SEMICONDUCTOR QUANTUM DOTS 
690 1 0 |a POLYMERS 
690 1 0 |a ACID ANHYDRIDE 
690 1 0 |a AMPHOPHILE 
690 1 0 |a AROMATIC AMINE 
690 1 0 |a CHLOROFORM 
690 1 0 |a FLUORESCENT DYE 
690 1 0 |a POLYMER 
690 1 0 |a QUANTUM DOT 
690 1 0 |a ANISOTROPY 
690 1 0 |a AQUEOUS SOLUTION 
690 1 0 |a ARTICLE 
690 1 0 |a BLEACHING 
690 1 0 |a CONFORMATION 
690 1 0 |a CONJUGATION 
690 1 0 |a CONTROLLED STUDY 
690 1 0 |a DENSITY 
690 1 0 |a ENERGY TRANSFER 
690 1 0 |a FLUORESCENCE SPECTROSCOPY 
690 1 0 |a GEL PERMEATION CHROMATOGRAPHY 
690 1 0 |a MICELLE 
690 1 0 |a PHOTOCHEMISTRY 
690 1 0 |a PHOTON 
690 1 0 |a QUANTUM YIELD 
690 1 0 |a SUSPENSION 
690 1 0 |a SYNTHESIS 
690 1 0 |a ULTRAVIOLET IRRADIATION 
690 1 0 |a FLUORESCENCE RESONANCE ENERGY TRANSFER 
690 1 0 |a KINETICS 
690 1 0 |a NANOPARTICLES 
690 1 0 |a POLYMERS 
690 1 0 |a QUANTUM DOTS 
690 1 0 |a SOLVENTS 
690 1 0 |a SPECTROPHOTOMETRY, ULTRAVIOLET 
650 1 7 |2 spines  |a COLOR 
700 1 |a Giordano, L. 
700 1 |a Azcárate, J.C. 
700 1 |a Jovin, T.M. 
700 1 |a Jares-Erijman, E.A. 
773 0 |d 2013  |g v. 135  |h pp. 3208-3217  |k n. 8  |p J. Am. Chem. Soc.  |x 00027863  |w (AR-BaUEN)CENRE-19  |t Journal of the American Chemical Society 
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856 4 0 |u https://doi.org/10.1021/ja3117813  |y DOI 
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